Creating a new electrode material of supercapacitors from the waste multi-walled carbon nanotubes | |
Chen, Yong; Xu, Cheng; Zhao, Jiang; Huang, Jiandi; Xu, Hui; Gou, Guojun | |
2020-01-10 | |
发表期刊 | ELECTROCHIMICA ACTA |
ISSN | 0013-4686 |
卷号 | 330 |
摘要 | Many adsorbents are discarded after removing pollutants, which always re-contaminateenvironment due to a release of pollutants again. The purpose of this study is to reuse the waste multi-walled carbon nanotubes (MWCNTs) who remove methylene blue (MB) from waste water as electrode material of supercapacitor. Herein, with a combination of polypyrrole (PPy), MWCNTs/MB/PPy composites are synthesized via chemical in-situ polymerization. The structure tests of the composites indicate that the surface property of MWCNTs, after adsorbing MB, is changed from hydrophobic to hydrophilic. Additionally, cyclic voltammetry (CV), galvanostatic charge-discharge (GCD), and electrochemical impedance spectrum (EIS) tests in three-electrode system demonstrate that at a current density of 5 mA cm(-2), the specific capacitance of MWCNTs/MB/PPy composites is 446 F g(-1). This result is higher than that of PPy and MWCNTs/PPy composites due to an extra pseudo-capacitance provided by MB. Moreover, a symmetric supercapacitor of MWCNTs/MB/PPy composites is assembled to successfully light a light emitting diodes (LED), which powerfully reveals the potential application of MWCNTs/MB/PPy composites. Obviously, the waste MWCNTs can be reused, meaning the dyes adsorbed on MWCNTs have no chance to pollute the environment again. (C) 2019 Elsevier Ltd. All rights reserved. |
关键词 | Adsorption Waste MWCNTs MWCNTs/MB/PPy composites Specific capacitance Symmetric supercapacitor |
DOI | 10.1016/j.electacta.2019.135237 |
收录类别 | SCI ; SCIE |
语种 | 英语 |
资助项目 | National Natural Science Foundations of China[51663014][51503092][51763015] ; Natural Science Foundation of Gansu Province[2017GS10857] |
WOS研究方向 | Electrochemistry |
WOS类目 | Electrochemistry |
WOS记录号 | WOS:000501468400018 |
出版者 | PERGAMON-ELSEVIER SCIENCE LTD |
EI入藏号 | 20194907788255 |
EI主题词 | Multiwalled carbon nanotubes (MWCN) |
EI分类号 | 444 Water Resources - 452.4 Industrial Wastes Treatment and Disposal - 701.1 Electricity: Basic Concepts and Phenomena - 761 Nanotechnology - 801.4.1 Electrochemistry - 802.3 Chemical Operations - 804.1 Organic Compounds - 815.1.1 Organic Polymers |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | https://ir.lut.edu.cn/handle/2XXMBERH/64235 |
专题 | 石油化工学院 |
通讯作者 | Chen, Yong; Xu, Hui |
作者单位 | Lanzhou Univ Technol, Coll Petrochem Engn, Lanzhou 730050, Gansu, Peoples R China |
第一作者单位 | 石油化工学院 |
通讯作者单位 | 石油化工学院 |
第一作者的第一单位 | 石油化工学院 |
推荐引用方式 GB/T 7714 | Chen, Yong,Xu, Cheng,Zhao, Jiang,et al. Creating a new electrode material of supercapacitors from the waste multi-walled carbon nanotubes[J]. ELECTROCHIMICA ACTA,2020,330. |
APA | Chen, Yong,Xu, Cheng,Zhao, Jiang,Huang, Jiandi,Xu, Hui,&Gou, Guojun.(2020).Creating a new electrode material of supercapacitors from the waste multi-walled carbon nanotubes.ELECTROCHIMICA ACTA,330. |
MLA | Chen, Yong,et al."Creating a new electrode material of supercapacitors from the waste multi-walled carbon nanotubes".ELECTROCHIMICA ACTA 330(2020). |
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