Fe3O4/PPy-Coated Superhydrophilic Polymer Porous Foam: A Double Layered Photothermal Material with a Synergistic Light-to-Thermal Conversion Effect toward Desalination
He, Jingxian1,2; Liu, Fang1,2; Xiao, Chaohu1; Sun, Hanxue1; Li, Jiyan1; Zhu, Zhaoqi1; Liang, Weidong1; Li, An1
2021-10-26
发表期刊LANGMUIR
ISSN0743-7463
卷号37期号:42页码:12397-12408
摘要Solar steam generation has been considered as one of the most promising strategies for production of fresh water using renewable solar energy. Herein, we prepared a polymer porous foam (HPSS) by a facile hydrothermal method. The HPSS presents a superhydrophilic wettability, an interpenetrating macro-porous structure, and low thermal conductivity, which can well satisfy the criteria as an ideal candidate for photothermal materials. The HPSS/Fe3O4/PPy (polypyrrole) evaporator, of which a Fe3O4/PPy binary optical system served as a light absorption layer and HPSS was used as a porous substrate, was constructed through in situ growth of Fe3O4 particles followed by interfacial polymerization of PPy on the surface of HPSS. HPSS/Fe3O4/PPy shows an excellent light absorption capacity (92%) and photo- thermal conversion performance, with the solar energy conversion efficiency reaching up to 94.7% under 1 sun irradiation, which is much higher than that of HPSS/PPy (84.8%) composed of a unitary PPy light absorption layer. Interestingly, the presence of Fe3O4 particles could make directional migration in a magnetic field possible, thus facilitating its recovery as a self-floating solar generator in an open water area. Moreover, the HPSS/Fe3O4/PPy evaporator displays outstanding salt resistance properties and stability in various saline solutions, thus having great potential in practical desalination.
DOI10.1021/acs.langmuir.1c02013
收录类别SCIE
语种英语
WOS研究方向Chemistry ; Materials Science
WOS类目Chemistry, Multidisciplinary ; Chemistry, Physical ; Materials Science, Multidisciplinary
WOS记录号WOS:000711763600016
出版者AMER CHEMICAL SOC
来源库WOS
引用统计
被引频次:16[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符https://ir.lut.edu.cn/handle/2XXMBERH/150069
专题石油化工学院
通讯作者Li, An
作者单位1.Lanzhou Univ Technol, Coll Petrochem Technol, Lanzhou 730050, Peoples R China;
2.Lanzhou City Univ, Sch Chem & Chem Engn, Lanzhou 730070, Peoples R China
第一作者单位石油化工学院
通讯作者单位石油化工学院
第一作者的第一单位石油化工学院
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He, Jingxian,Liu, Fang,Xiao, Chaohu,et al. Fe3O4/PPy-Coated Superhydrophilic Polymer Porous Foam: A Double Layered Photothermal Material with a Synergistic Light-to-Thermal Conversion Effect toward Desalination[J]. LANGMUIR,2021,37(42):12397-12408.
APA He, Jingxian.,Liu, Fang.,Xiao, Chaohu.,Sun, Hanxue.,Li, Jiyan.,...&Li, An.(2021).Fe3O4/PPy-Coated Superhydrophilic Polymer Porous Foam: A Double Layered Photothermal Material with a Synergistic Light-to-Thermal Conversion Effect toward Desalination.LANGMUIR,37(42),12397-12408.
MLA He, Jingxian,et al."Fe3O4/PPy-Coated Superhydrophilic Polymer Porous Foam: A Double Layered Photothermal Material with a Synergistic Light-to-Thermal Conversion Effect toward Desalination".LANGMUIR 37.42(2021):12397-12408.
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