Sonocatalytic degradation of Rhodamine B catalyzed by β-Bi2O3 particles under ultrasonic irradiation | |
Chen, Xuefu1,2; Dai, Jianfeng2; Shi, Gaofeng1; Li, Lan1; Wang, Guoying1; Yang, Hua2 | |
2016-03-01 | |
发表期刊 | Ultrasonics Sonochemistry |
ISSN | 13504177 |
卷号 | 29页码:172-177 |
摘要 | β-Bi2O3 particles were synthesized by a polyacrylamide sol-gel method. The sonocatalytic activity of β-Bi2O3 particles was evaluated by degrading Rhodamine B (RhB) under the ultrasonic irradiation, revealing that β-Bi2O3 particles exhibit a good sonocatalytic activity. The effects of various experimental factors including ultrasonic frequency (f), solution temperature (T), catalyst dosage (Ccatalyst) and initial RhB concentration (CRhB) on the sonocatalysis efficiency were investigated. The optimum conditions for sonocatalytic degradation of RhB are obtained to be f = 60 kHz, T = 40 °C, Ccatalyst = 3 g L-1, and CRhB = 5 mg L-1. The percentage degradation of RhB after sonocatalysis for 90 min is 98.7%. Detected by the photoluminescence technique that of using terephthalic acid as a probe molecule, hydroxyl radicals (OH) are found to be produced on the irradiated by β-Bi2O3 particles. Based on the experimental results, OH radicals are suggested to be the major active species which are responsible for the degradation reaction. © 2015 Published by Elsevier B.V. |
关键词 | Free radicals Irradiation Rhodium compounds Sol-gel process Sol-gels Ultrasonic applications Experimental factors Influencing factors OH radical Solution temperature Sonocatalytic Sonocatalytic degradation Ultrasonic frequency Ultrasound irradiation |
DOI | 10.1016/j.ultsonch.2015.08.010 |
收录类别 | EI ; SCIE |
语种 | 英语 |
WOS研究方向 | Acoustics ; Chemistry |
WOS类目 | Acoustics ; Chemistry, Multidisciplinary |
WOS记录号 | WOS:000366238000018 |
出版者 | Elsevier B.V. |
EI入藏号 | 20154101372413 |
EI主题词 | Bismuth compounds |
EI分类号 | 753.3 Ultrasonic Applications - 804 Chemical Products Generally - 812.3 Glass |
来源库 | Compendex |
分类代码 | 753.3 Ultrasonic Applications - 804 Chemical Products Generally - 812.3 Glass |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | https://ir.lut.edu.cn/handle/2XXMBERH/112601 |
专题 | 石油化工学院 理学院 |
通讯作者 | Dai, Jianfeng |
作者单位 | 1.Lanzhou Univ Technol, Coll Petrochem Technol, Lanzhou 730050, Peoples R China; 2.Lanzhou Univ Technol, State Key Lab Adv Proc & Recycling Nonferrous Met, Lanzhou 730050, Peoples R China |
第一作者单位 | 石油化工学院; 省部共建有色金属先进加工与再利用国家重点实验室 |
通讯作者单位 | 省部共建有色金属先进加工与再利用国家重点实验室 |
第一作者的第一单位 | 石油化工学院 |
推荐引用方式 GB/T 7714 | Chen, Xuefu,Dai, Jianfeng,Shi, Gaofeng,et al. Sonocatalytic degradation of Rhodamine B catalyzed by β-Bi2O3 particles under ultrasonic irradiation[J]. Ultrasonics Sonochemistry,2016,29:172-177. |
APA | Chen, Xuefu,Dai, Jianfeng,Shi, Gaofeng,Li, Lan,Wang, Guoying,&Yang, Hua.(2016).Sonocatalytic degradation of Rhodamine B catalyzed by β-Bi2O3 particles under ultrasonic irradiation.Ultrasonics Sonochemistry,29,172-177. |
MLA | Chen, Xuefu,et al."Sonocatalytic degradation of Rhodamine B catalyzed by β-Bi2O3 particles under ultrasonic irradiation".Ultrasonics Sonochemistry 29(2016):172-177. |
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