Three-Dimensional Interconnected Microporous Carbon Network Derived from Aniline Formaldehyde Resin/Sodium Polyacrylate Interpenetrating Polymer Networks (AF/PAAS IPNs) with Controllable Porosity for Supercapacitors
Ma, Yan-Dong1; Chen, Xi-Wen1; Kong, Ling-Bin1,2
2019-09
Source PublicationACS APPLIED ENERGY MATERIALS
ISSN2574-0962
Volume2Issue:9Pages:6440-6452
AbstractA facile strategy for the synthesis of three-dimensional nitrogen-doped microporous carbon (MC-IPNx) is reported here. We adopt the advantages of cross-linking individually of interpenetrating polymer networks to synthesize porous carbon with well-controlled micropores (similar to 0.6 nm) and interconnected pores by one-step carbonization of aniline formaldehyde resin/sodium polyacrylate interpenetrating polymer networks (AF/PAAS IPNs), a radically different approach that allows AF/PAAS IPNs to be directly converted to nitrogen-doped microporous carbon (MC-IPNx) without any pretreatment. Due to the interpenetrating pores and abundant porosity, MC-IPNx acquired a high specific surface area (1275 m(2) g(-1)), which reveals remarkable specific capacity (223 F g(-1) at a current density of 1 A g(-1)) and superb capacity retention (80% retention in a current density within the range 0.5-10 A g(-1)). The unique pore structure of MC-IPNx provides an innovative idea for the control of pore size, and advanced electrochemical performance indicates its application prospects.
Keywordinterpenetrating polymer networks microporous carbon controllable pore size supercapacitors electrochemical performance
DOI10.1021/acsaem.9b01044
Indexed BySCI
Language英语
Funding ProjectNational Natural Science Foundation of China[51762031] ; Foundation for Innovation Groups of Basic Research in Gansu Province[1606RJIA322]
WOS Research AreaChemistry ; Energy & Fuels ; Materials Science
WOS SubjectChemistry, Physical ; Energy & Fuels ; Materials Science, Multidisciplinary
WOS IDWOS:000487770000038
PublisherAMER CHEMICAL SOC
Document Type期刊论文
Identifierhttp://ir.lut.edu.cn/handle/2XXMBERH/64272
Collection省部共建有色金属先进加工与再利用国家重点实验室
材料科学与工程学院
Corresponding AuthorKong, Ling-Bin
Affiliation1.Lanzhou Univ Technol, State Key Lab Adv Proc & Recycling Nonferrous Met, Lanzhou 730050, Gansu, Peoples R China
2.Lanzhou Univ Technol, Sch Mat Sci & Engn, Lanzhou 730050, Gansu, Peoples R China
First Author AffilicationState Key Laboratory Of Gansu Advanced Non-Ferrous Metal Materials
Corresponding Author AffilicationState Key Laboratory Of Gansu Advanced Non-Ferrous Metal Materials;  Coll Mat Sci & Engn
First Signature AffilicationState Key Laboratory Of Gansu Advanced Non-Ferrous Metal Materials
Recommended Citation
GB/T 7714
Ma, Yan-Dong,Chen, Xi-Wen,Kong, Ling-Bin. Three-Dimensional Interconnected Microporous Carbon Network Derived from Aniline Formaldehyde Resin/Sodium Polyacrylate Interpenetrating Polymer Networks (AF/PAAS IPNs) with Controllable Porosity for Supercapacitors[J]. ACS APPLIED ENERGY MATERIALS,2019,2(9):6440-6452.
APA Ma, Yan-Dong,Chen, Xi-Wen,&Kong, Ling-Bin.(2019).Three-Dimensional Interconnected Microporous Carbon Network Derived from Aniline Formaldehyde Resin/Sodium Polyacrylate Interpenetrating Polymer Networks (AF/PAAS IPNs) with Controllable Porosity for Supercapacitors.ACS APPLIED ENERGY MATERIALS,2(9),6440-6452.
MLA Ma, Yan-Dong,et al."Three-Dimensional Interconnected Microporous Carbon Network Derived from Aniline Formaldehyde Resin/Sodium Polyacrylate Interpenetrating Polymer Networks (AF/PAAS IPNs) with Controllable Porosity for Supercapacitors".ACS APPLIED ENERGY MATERIALS 2.9(2019):6440-6452.
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