Preparation of heterogeneous Fenton catalyst Fe/organo-attapulgite and its performance in sodium humate degradation
Zhang, Ting; Liu, Jin; Chen, Minmin; Wang, Yi
2018-03
发表期刊DESALINATION AND WATER TREATMENT
ISSN1944-3994
卷号107页码:91-99
摘要A novel heterogeneous Fenton catalyst Fe/organo-attapulgite (Fe/OATP) was prepared by introducing nano-Fe into organic modified attapulgite with redox method. The new catalyst was characterized by XRD, IR and SEM, and a series of experiments were conducted for investigating the influences of pH value, catalyst dosage, hydrogen peroxide concentration, reaction temperature and initial concentration of HA-Na solution on the degradation ratios of HA-Na in Fe/OATP/H2O2 heterogeneous Fenton system. Through a number of degradation experiments under various conditions, the results showed that the removal ratio of HA-Na can reach more than 97% at the condition of pH value 8, the reaction temperature 70 degrees C, the initial HA-Na concentration 100 mg/L, the catalysts dosage 10 g/L, and the H2O2 concentration 78.4 mmol/L. According to the results of dynamics experiments, the degradation of HA-Na followed the first-order kinetics. Fe/OATP catalyst has a wide pH range in heterogeneous Fenton reaction and can be reused for many runs with good capacity of HA-Na degradation.
关键词Attapulgite (ATP) Heterogeneous Fenton catalyst Degradation HA-Na
DOI10.5004/dwt.2018.22111
收录类别SCI ; SCIE
语种英语
资助项目National Natural Science Foundation of China[51302123]
WOS研究方向Engineering ; Water Resources
WOS类目Engineering, Chemical ; Water Resources
WOS记录号WOS:000445119300010
出版者DESALINATION PUBL
引用统计
被引频次:1[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符https://ir.lut.edu.cn/handle/2XXMBERH/32753
专题石油化工学院
通讯作者Zhang, Ting
作者单位Lanzhou Univ Technol, Dept Petrochem Engn, Lanzhou 730050, Gansu, Peoples R China
第一作者单位兰州理工大学
通讯作者单位兰州理工大学
第一作者的第一单位兰州理工大学
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GB/T 7714
Zhang, Ting,Liu, Jin,Chen, Minmin,et al. Preparation of heterogeneous Fenton catalyst Fe/organo-attapulgite and its performance in sodium humate degradation[J]. DESALINATION AND WATER TREATMENT,2018,107:91-99.
APA Zhang, Ting,Liu, Jin,Chen, Minmin,&Wang, Yi.(2018).Preparation of heterogeneous Fenton catalyst Fe/organo-attapulgite and its performance in sodium humate degradation.DESALINATION AND WATER TREATMENT,107,91-99.
MLA Zhang, Ting,et al."Preparation of heterogeneous Fenton catalyst Fe/organo-attapulgite and its performance in sodium humate degradation".DESALINATION AND WATER TREATMENT 107(2018):91-99.
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