One-Pot Hydrothermal Synthesis of Solution-Processable MoS2/PEDOT:PSS Composites for High-Performance Supercapacitors | |
Chao, Yunfeng1; Ge, Yu1; Chen, Zhiqi1; Cui, Xiaoling2; Zhao, Chen3; Wang, Caiyun1; Wallace, Gordon G.1 | |
2021-02-17 | |
发表期刊 | ACS APPLIED MATERIALS & INTERFACES |
ISSN | 1944-8244 |
卷号 | 13期号:6页码:7285-7296 |
摘要 | It is challenging to hydrothermally synthesize solution-processable MoS2, as the strong van der Waals force between MoS2 nanosheets induces self-assembly of agglomerates. Here, we introduce poly(3,4-ethylenedioxythiophene): poly(styrenesulfonate) (PE-DOT:PSS) into the precursor to impede aggregate formation in the hydrothermal process. A hybrid MoS2/PEDOT:PSS (MP) hydrogel is formed due to the electrostatic interactions between the negatively charged MoS2 and positively charged PEDOT chains. This hydrogel can be easily dispersed in water for subsequent solution processing such as vacuum filtration to form free-standing flexible films or extrusion 3D printing to create novel patterns. The MP film with a fracture strength of 18.59 MPa displays excellent electrochemical performance in both aqueous Na2SO4 electrolyte (474 mF cm(-2)) and solid-state PVA-H3PO4 electrolyte (360 mF cm(-2)). Flexibility and robustness can be evidenced by high capacitance retention rates of 94 and 89% after being repeatedly bent to 180 degrees for 5000 cycles in aqueous and solid-state electrolytes, respectively. |
关键词 | MoS2/PEDOT:PSS composites hydrothermal method hybrid structure solution processable supercapacitors |
DOI | 10.1021/acsami.0c21439 |
收录类别 | SCIE |
语种 | 英语 |
WOS研究方向 | Science & Technology - Other Topics ; Materials Science |
WOS类目 | Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary |
WOS记录号 | WOS:000621051200029 |
出版者 | AMER CHEMICAL SOC |
EI入藏号 | 20210709911751 |
EI主题词 | Hydrothermal synthesis |
EI分类号 | 708.2 Conducting Materials - 745.1.1 Printing Equipment - 801.4 Physical Chemistry - 802.2 Chemical Reactions - 802.3 Chemical Operations - 803 Chemical Agents and Basic Industrial Chemicals - 804 Chemical Products Generally - 804.2 Inorganic Compounds |
来源库 | WOS |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | https://ir.lut.edu.cn/handle/2XXMBERH/147459 |
专题 | 石油化工学院 |
通讯作者 | Wang, Caiyun; Wallace, Gordon G. |
作者单位 | 1.Univ Wollongong, ARC Ctr Excellence Electromat Sci, Intelligent Polymer Res Inst, AIIM Facil, Innovat Campus, Wollongong, NSW 2522, Australia; 2.Lanzhou Univ Technol, Coll Petrochem Technol, Lanzhou 730050, Peoples R China; 3.Guangdong Univ Technol, Sch Mat & Energy, Guangzhou 510006, Peoples R China |
推荐引用方式 GB/T 7714 | Chao, Yunfeng,Ge, Yu,Chen, Zhiqi,et al. One-Pot Hydrothermal Synthesis of Solution-Processable MoS2/PEDOT:PSS Composites for High-Performance Supercapacitors[J]. ACS APPLIED MATERIALS & INTERFACES,2021,13(6):7285-7296. |
APA | Chao, Yunfeng.,Ge, Yu.,Chen, Zhiqi.,Cui, Xiaoling.,Zhao, Chen.,...&Wallace, Gordon G..(2021).One-Pot Hydrothermal Synthesis of Solution-Processable MoS2/PEDOT:PSS Composites for High-Performance Supercapacitors.ACS APPLIED MATERIALS & INTERFACES,13(6),7285-7296. |
MLA | Chao, Yunfeng,et al."One-Pot Hydrothermal Synthesis of Solution-Processable MoS2/PEDOT:PSS Composites for High-Performance Supercapacitors".ACS APPLIED MATERIALS & INTERFACES 13.6(2021):7285-7296. |
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